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Libby and graduate student Ernest Anderson (1920–2013) calculated the mixing of carbon across these different reservoirs, particularly in the oceans, which constitute the largest reservoir.
Their results predicted the distribution of carbon-14 across features of the carbon cycle and gave Libby encouragement that radiocarbon dating would be successful.
In a system where carbon-14 is readily exchanged throughout the cycle, the ratio of carbon-14 to other carbon isotopes should be the same in a living organism as in the atmosphere.
However, the rates of movement of carbon throughout the cycle were not then known.
Further research by Libby and others established its half-life as 5,568 years (later revised to 5,730 ± 40 years), providing another essential factor in Libby’s concept.
Korff predicted that the reaction between these neutrons and nitrogen-14, which predominates in the atmosphere, would produce carbon-14, also called radiocarbon.
Libby cleverly realized that carbon-14 in the atmosphere would find its way into living matter, which would thus be tagged with the radioactive isotope.
Theoretically, if one could detect the amount of carbon-14 in an object, one could establish that object’s age using the half-life, or rate of decay, of the isotope.
In 1946, Libby proposed this groundbreaking idea in the journal Physical Review.